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3D printed optimized electrodes for electrochemical flow reactors

delete2024-09-30
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OA
AI
J
Jonathan T. Davis
B
Buddhinie Srimali Jayathilake
S
Swetha Chandrasekaran
J
Jonathan J. Wong
J
Joshua R. Deotte
S
Sarah E. Baker
V
V. A. Beck
E
Eric B. Duoss
M
Marcus A. Worsley
T
Tiras Y. Lin *
DOI:10.1038/s41598-024-71765-wdelete
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摘要

摘要

En 中文
Recent advances in 3D printing have enabled the manufacture of porous electrodes which cannot be machined using traditional methods. With micron-scale precision, the pore structure of an electrode can now be designed for optimal energy efficiency, and a 3D printed electrode is not limited to a single uniform porosity. As these electrodes scale in size, however, the total number of possible pore designs can be intractable; choosing an appropriate pore distribution manually can be a complex task. To address this challenge, we adopt an inverse design approach. Using physics-based models, the electrode structure is optimized to minimize power losses in a flow reactor. The computer-generated structure is then printed and benchmarked against homogeneous porosity electrodes. We show how an optimized electrode decreases the power requirements by 16% compared to the best-case homogeneous porosity. Future work could apply this approach to flow batteries, electrolyzers, and fuel cells to accelerate their design and implementation.
Keyword:
Optimized electrodes
Inverse design
Electrochemical reactors
Flow batteries
3D Printing
Porous electrodes
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期刊

Scientific Reports 封面图
Scientific Reports
IF:
3.9
论文数:
27.9W
被引数:
83.5W

机构

U
united states department of energy (doe)
学者数:
11.3W
论文数: 9.6W
被引数: 246
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