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4D Printed Shape-Memory Elastomer for Thermally Programmable Soft Actuators

delete2023-08-18
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OA
AI
Q
Qingchuan Song
Y
Yunong Chen
V
Viacheslav Slesarenko
P
Pang Zhu
A
Ahmed Hamza
P
Peilong Hou
D
Dorothea Helmer
F
Frederik Kotz *
B
Bastian E. Rapp
DOI:10.1021/acsami.3c07436delete
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摘要

摘要

En 中文
Polymeric shape-memory elastomers can recover to a permeantshapefrom any programmed deformation under external stimuli. They are mostlycross-linked polymeric materials and can be shaped by three-dimensional(3D) printing. However, 3D printed shape-memory polymers so far onlyexhibit elasticity above their transition temperature, which resultsin their programmed shape being inelastic or brittle at lower temperatures.To date, 3D printed shape-memory elastomers with elasticity both belowand above their transition temperature remain an elusive goal, whichlimits the application of shape-memory materials as elastic materialsat low temperatures. In this paper, we printed, for the first time,a custom-developed shape-memory elastomer based on polyethylene glycolusing digital light processing, which possesses elasticity and stretchabilityin a wide temperature range, below and above the transition temperature.Young's modulus in these two states can vary significantly,with a difference of up to 2 orders of magnitude. This marked differencein Young's modulus imparts excellent shape-memory propertiesto the material. The difference in Young's modulus at differenttemperatures allows for the programming of the pneumatic actuatorsby heating and softening specific areas. Consequently, a single actuatorcan exhibit distinct movement modes based on the programming processit undergoes.
Keyword:
4D printing
shape memory polymers
shape memoryelastomers
digital light processing
programmablepneumatic actuators
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期刊

ACS Applied Materials and Interfaces 封面图
ACS Applied Materials and Interfaces
IF:
8.2
论文数:
6.1W
被引数:
38.7W

机构

U
University of Freiburg
学者数:
3.3W
论文数: 2.4W
被引数: 3.4W
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