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An analytical solution to multi-component NAPL dissolution equations
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DOI：10.1016/j.advwatres.2006.05.007.png)
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This note presents a novel method for determining the changing composition of a multi-component NAPL body dissolving into moving groundwater, and the consequent changes in the aqueous phase solute concentrations in the surrounding pore water. A canonical system of coupled non-linear governing equations is derived which is suitable for representation of both pooled and residual configurations, and this is solved. Whereas previous authors have handled such problems numerically, it is shown that these governing equations succumb to analytical solution. By a suitable substitution, the equations become decoupled, and the problem collapses to a single first-order equation. The final result is expressed implicitly, with time as a function of the number of moles of the least soluble component, m(1). The number of moles of each other component is expressed explicitly in terms of m(1). It is shown that the time-nil relationship has a well behaved inverse. An example is given in which the analytic solution is verified against traditional finite difference analysis, and its computational efficiency is shown. (C) 2006 Elsevier Ltd. All rights reserved.
Keyword:
NAPL
multi-component
dissolution
solubility
analytical solution
Raoult's law
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