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Catalyst Design with Atomic Layer Deposition
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DOI：10.1021/cs501862h.png)
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摘要
En 中文
Atomic layer deposition (ALD) has emerged as an interesting tool for the atomically precise design and synthesis of catalytic materials Herein, we discuss examples in which the atomic precision has been used to elucidate reaction mechanisms and catalyst structure property relationships by creating materials With a Controlled distribution of size, composition, and active site We highlight ways ALD has been utilized to design catalysts with improved activity, selectivity, and stability under a variety of conditions (e.g., high temperature, gas and liquid phase, and corrosive environments). In addition, due to the flexibility and control of structure and composition, ALD can create myriad catalytic structures (e.g., high surface area oxides, metal nanoparticles, bimetallic nanoparticles, bifunctional catalysts, controlled microenvironments, etc.) that consequently possess applicability for a wide range of chemical reactions (e.g., CO2 conversion, electrocatalysis, photocatalytic and thermal water splitting, methane conversion, ethane and propane dehydrogenation, and biomass conversion). Finally, the outlook for ALD-derived catalytic materials is discussed, with emphasis on the pending challenges as well as areas of significant potential for building scientific insight and achieving practical impacts.
Keyword:
atomic layer deposition
ALD
catalyst overcoating
metal nanoparticles
bimetallic nanoparticles
controlled synthesis
catalyst design
mechanism elucidation
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IF:
13.1
论文数:
1.6W
被引数:
15.0W
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