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摘要
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A strong helicity dependence of reconstruction of attosecond bursts by beating of two-photon transitions (RABBITT) with circularly polarized XUV and IR pulses was reported by Han et al. [Nat. Phys. 19, 1649 (2023) and arXiv:2302.04137]. They attributed a circular dichroic phase in RABBITT to the helical structure of the photoelectron wave packets in the final state. We exploit this effect to determine the magnitude and phase of two-photon XUV + IR ionization amplitudes. In s-electron targets (H, He, Li), such a determination is fully ab initio and requires no further approximations. In heavier noble gases like Ar, characterization of two-photon ionization amplitudes can be made from the circular dichroic phase with minimal and very realistic assumptions.
期刊
IF:
4.2
论文数:
7.6K
被引数:
2.7W
机构
引用论文
Determining the polarization state of an extreme ultraviolet free-electron laser beam using atomic circular dichroism
NATURE COMMUNICATIONS
IF15.7

