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Decrease in Nucleated Particles and Cloud Condensation Nuclei Observed across a Range of Environments

delete2026-04-27
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OA
AI
D
Do-Hyeon Park
P
Paolo Laj
E
Elisabeth Andrews
C
Clémence Rose
A
Angela Benedetti
M
Markku Kulmala
I
Inés Zabala
E
Erik Ahlberg
A
Andrés Alástuey
E
Eija Asmi
O
Olaf Bath
T
Tak Wai Chan
J
Jin-soo Choi
M
Martine Collaud Coen
S
Sébastien Conil
S
Sebastiao Martins Dos Santos
K
Konstantinos Eleftheriadis
M
Markus Fiebig
M
Maria I. Gini
A
A. Gannet Hallar
A
Antti Hyvärinen
L
Leena Järvi
N
Nikos Kalivitis
M
Melita Keywood
J
Jeong Eun Kim
S
Sumin Kim
J
Jenni Kontkanen
G
Giorgos Kouvarakis
A
Adam Kristensson
C
Chongai Kuang
M
Meehye Lee
H
Heikki Lihavainen
Y
Yong Lin
C
Chris Lunder
A
Atsushi Matsuki
O
Olga L. Mayol-Bracero
M
Maik Merkel
N
Nikolaos Mihalopoulos
C
Cathrine Lund Myhre
J
Jin-soo Park
M
Minsu Park
R
Rokjin J. Park
T
Tuukka Petäja
J
Jean-Philippe Putaud
A
Andreas Schwerin
K
Karine Sellegri
E
Erik Swietlicki
T
Thomas Tuch
P
Peter Tunved
V
Ville Vakkari
P
Paolo Villani
S
Stergios Vratolis
K
Kay Weinhold
A
Alfred Wiedensohler
Y
Young Jun Yoon
S
Seong Soo Yum
V
Vladimir Zdimal
J
John A. Ogren
S
Sang‐Woo Kim *
DOI：10.1021/acs.est.5c18035delete
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摘要

摘要

En 中文
理解新粒子生成（NPF）和纳米粒子的归宿至关重要，因为它们与空气质量、云形成和气候密切相关。这些影响因多样的气溶胶来源及其相对较短的大气寿命而在空间和时间上存在差异。在此，我们利用来自37个站点（主要来自全球大气观测（GAW）站）的经过质量控制的质量浓度分布（PNSD）和云凝结核（CCN）数据，对多种观测环境中与NPF相关的成核模式粒子和云凝结核浓度的长期趋势进行了综合分析。我们发现，在大多数站点类型中，NPF的发生和成核粒子浓度均呈现下降的十年趋势，其中城市地区的下降最为显著。我们观察到CCN浓度和成核模式粒子同时减少，这表明新生成粒子可能是CCN的潜在来源。进而表明，通过改变云滴形成的气溶胶-云相互作用，可以间接影响云微物理性质和辐射效应。这些发现表明，人为排放的减少可能会影响气溶胶-云相互作用的气候强迫潜力，这对未来气候预测具有重要意义。
Keyword:
Aerosols
Climate
Condensation
Nanoparticles
Redox reactions
new particle formation
particle number size distribution
cloud condensation nuclei
aerosol−cloud interactions
air quality regulations

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