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Electrotunable liquid sulfur microdroplets

delete2020-01-30
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周光敏 封面图
周光敏 (Guangmin Zhou)
A
Ankun Yang
Y
Yifei Wang
高国平 封面图
高国平 (Guoping Gao)
A
Allen Pei
Y
Yu, Xiaoyun
Y
Yangying Zhu
L
Linqi Zong
B
Bofei Liu
J
Jinwei Xu
刘念 封面图
刘念 (Nian Liu)
J
Jinsong Zhang
Y
Yanxi Li
L
Lin‐Wang Wang
H
Harold Y. Hwang
M
Mark L. Brongersma
S
Steven Chu
Y
Yi Cui *
DOI:10.1038/s41467-020-14438-2delete
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摘要

摘要

En 中文
Manipulating liquids with tunable shape and optical functionalities in real time is important for electroactive flow devices and optoelectronic devices, but remains a great challenge. Here, we demonstrate electrotunable liquid sulfur microdroplets in an electrochemical cell. We observe electrowetting and merging of sulfur droplets under different potentiostatic conditions, and successfully control these processes via selective design of sulfiphilic/sulfiphobic substrates. Moreover, we employ the electrowetting phenomena to create a microlens based on the liquid sulfur microdroplets and tune its characteristics in real time through changing the shape of the liquid microdroplets in a fast, repeatable, and controlled manner. These studies demonstrate a powerful in situ optical battery platform for unraveling the complex reaction mechanism of sulfur chemistries and for exploring the rich material properties of the liquid sulfur, which shed light on the applications of liquid sulfur droplets in devices such as microlenses, and potentially other electrotunable and optoelectronic devices. Manipulating liquids with tunable shape and optical functionalities in real time remains a great challenge. Here, the authors demonstrate electrotunable liquid sulfur microdroplets in an electrochemical cell and tune its characteristics in a fast, repeatable, and controlled manner.
Keyword:
TOTAL-ENERGY CALCULATIONS
NUCLEATION
DENSITY
SUPERHYDROPHOBICITY
SURFACES
NUCLEUS
DESIGN
GROWTH
WORK
SIZE
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Nature Communications 封面图
Nature Communications
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15.7
论文数:
9.3W
被引数:
91.2W

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tsinghua university
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被引数: 137
S
Stanford University
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论文数: 8.2W
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Lawrence Berkeley National Laboratory
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