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Harnessing Disorder for High-Performance Solid-State Electrolytes

delete2025-07-14
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PRE
AI
Z
Zhongkai Guo
Q
Qingkun Zhu
T
Tianming Chen
J
Jiping Sun
L
Lishun Bai
Y
Yue Liu
H
Huidong Niu
Y
Ying He
F
Feiyan Yu
K
Kuhang Liu
C
Chengjun Liu
J
Jinhao Xu
李
李四杰 (Sijie Li) *
Z
Zhi Chang *
DOI:10.1021/acsnano.5c07439delete
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摘要

摘要

En 中文
固态电解质(SSEs)已作为传统液态电解质的变革性替代方案出现,在解决关键挑战的同时,实现了更安全的运行环境、更宽的操作电压窗口以及更高能量密度的电池。高离子电导率无机固态电解质(HC-ISEs),如LGPS(Li10GeP2S12),表现出优异的离子电导率,但存在界面不稳定性、晶界电阻、与锂金属阳极兼容性差以及环境敏感性等问题。近期研究表明,通过阳离子位点无序化、非晶相集成和玻璃-陶瓷结构不规则性实现的工程无序,能够优化离子扩散通道、降低界面电阻并提升电化学稳定性。本综述系统分析了受控无序如何提升HC-ISEs的性能,探讨了定制无序结构的策略,并强调了其在实现高可靠性、高能量密度下一代固态电池中的关键作用。
Keyword:
solid-state electrolytes
high ionic conductivity
engineered disorder
lithium metal anode
next-generation batteries

期刊

ACS Nano 封面图
ACS Nano
IF:
16
论文数:
2.7W
被引数:
25.6W

机构

C
Central South University
学者数:
10.0W
论文数: 7.2W
被引数: 10.9W
引用论文

引用论文

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