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High-harmonic generation in amorphous solids

delete2017-09-28
delete174
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OA
AI
Y
Yong Sing You
Y
Yanchun Yin
Y
Yi Wu
A
Andrew Chew
X
Xiaoming Ren
F
Fengjiang Zhuang
S
Shima Gholam-Mirzaei
C
Chini, Michael
Z
Zenghu Chang
S
Shambhu Ghimire *
DOI:10.1038/s41467-017-00989-4delete
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摘要

摘要

En 中文
High-harmonic generation in isolated atoms and molecules has been widely utilized in extreme ultraviolet photonics and attosecond pulse metrology. Recently, high-harmonic generation has been observed in solids, which could lead to important applications such as all-optical methods to image valance charge density and reconstruct electronic band structures, as well as compact extreme ultraviolet light sources. So far these studies are confined to crystalline solids; therefore, decoupling the respective roles of long-range periodicity and high density has been challenging. Here we report the observation of high-harmonic generation from amorphous fused silica. We decouple the role of long-range periodicity by comparing harmonics generated from fused silica and crystalline quartz, which contain the same atomic constituents but differ in long-range periodicity. Our results advance current understanding of the strong-field processes leading to high-harmonic generation in solids with implications for the development of robust and compact extreme ultraviolet light sources.
Keyword:
ULTRAVIOLET-RADIATION
SPECTROSCOPY
ELECTRONS
PULSES
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Nature Communications
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Stanford University
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SLAC National Accelerator Laboratory
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united states department of energy (doe)
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