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High-Q dark hyperbolic phonon-polaritons in hexagonal boron nitride nanostructures

delete2020-05-18
delete13
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OA
AI
G
Georg Ramer
M
Mohit Tuteja
J
Joseph R. Matson
M
Marcelo Davanço
T
Thomas G. Folland
A
Andrey V. Kretinin
T
Takashi Taniguchi
K
Kenji Watanabe
K
Kostya S. Novoselov
J
Joshua D. Caldwell
A
Andrea Centrone *
DOI:10.1515/nanoph-2020-0048delete
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Abstract

Abstract

En 中文
The anisotropy of hexagonal boron nitride (hBN) gives rise to hyperbolic phonon-polaritons (HPhPs), notable for their volumetric frequency-dependent propagation and strong confinement. For frustum (truncated nanocone) structures, theory predicts five, high-order HPhPs, sets, but only one set was observed previously with far-field reflectance and scattering-type scanning near-field optical microscopy. In contrast, the photothermal induced resonance (PTIR) technique has recently permitted sampling of the full HPhP dispersion and observing such elusive predicted modes; however, the mechanism underlying PTIR sensitivity to these wealdy-scattering modes, while critical to their understanding, has not yet been clarified. Here, by comparing conventional contact- and newly developed tapping-mode PTIR, we show that the PTIR sensitivity to those wealdy-scattering, high-Q (up to approximate to 280) modes is, contrary to a previous hypothesis, unrelated to the probe operation (contact or tapping) and is instead linked to PTIR ability to detect tip-launched dark, volumetrically-confined polaritons, rather than nanostructure-launched HPhPs modes observed by other techniques. Furthermore, we show that in contrast with plasmons and surface phonon-polaritons, whose Q-factors and optical cross-sections are typically degraded by the proximity of other nanostructures, the high-Q HPhP resonances are preserved even in high-density hBN frustum arrays, which is useful in sensing and quantum emission applications.
Keywords:
dark modes
hexagonal boron nitride
high-Q
hyperbolic phonon polariton
PTIR
s-SNOM
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Nanophotonics cover
Nanophotonics
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vanderbilt university
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national institute of standards & technology (nist) - usa
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University of Manchester
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