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Hot pressing a high loading FeS2 all-solid-state composite cathode improves initial cycle performance

delete2024-06-27
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PRE
AI
T
Thomas A. Yersak *
H
Hernando J. Gonzalez Malabet
M
Mei Cai
DOI:10.1007/s10008-024-05989-1delete
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摘要

摘要

En 中文
本研究报告了在240 ℃ 和47 MPa下热压高负载 (9.375 mg cm(-2); > 5 mAh cm(-2)) 全固态FeS2复合阴极改善了初始循环性能。在25摄氏度下,冷压电池提供的容量可忽略不计,而热压电池提供的容量为332 mAh g(-1) (2.34 mAh cm(-2))。在60 ℃ 下,冷压电池输送666 mAh g(-1) (4.70 mAh cm(-2)),而热压电池输送782 mAh g(-1) (5.52 mAh cm(-2))。热压阴极复合材料具有20% 的孔隙率,而冷压阴极复合材料具有30% 的孔隙率。初始放电容量的增加归因于硫化物固态电解质 (SSE) 颗粒之间以及SSE和FeS2活性材料颗粒之间更好的固-固界面接触。由于锂化fes2的膨胀产生的应力,在延长的循环后发生电池故障。死后阴极复合材料的FIBSEM横截面成像显示出水平裂纹,表明由于电极膨胀而导致的电极分层。
Keyword:
All-solid-state battery
FeS2
Composite
Cathode
Consolidation
Hot pressing

期刊

Journal of Solid State Electrochemistry 封面图
Journal of Solid State Electrochemistry
IF:
2.6
论文数:
2.2K
被引数:
1.0W

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