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Hydrogen-bonded Complex-based Frameworks for Stable Lithium Storage
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DOI：10.1002/asia.202300310.png)
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摘要
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Metal-complex-based materials for lithium storage have attracted great interest due to their highly designable structures with multiple active sites and well-defined lithium transport pathways. Their cycling and rate performances, however, are still constrained by structural stability and electrical conductivity. Herein, we present two hydrogen-bonded complex-based frameworks with excellent lithium storage capability. Multiple hydrogen bonds among the mononuclear molecules result in three-dimensional frameworks that are stable in electrolyte. The origin of the remarkable lithium storage performance of this family was revealed through kinetic analysis and DFT calculations.
Keyword:
Lithium-ion battery
Metal-organic complex
Hydrogen-bonded framework
Dimensional design
期刊
C
IF:
3.3
论文数:
8.2K
被引数:
1.7W
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