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Interatomic and intermolecular decay processes in quantum fluid clusters

delete2024-11-19
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PRE
AI
A
Aaron LaForge
L
Ltaief Ben Ltaief
S
S. R. Krishnan
N
Nicolas Sisourat
M
M. Mudrich *
DOI:10.1088/1361-6633/ad8fbbdelete
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摘要

摘要

En 中文
In this comprehensive review, we explore interatomic and intermolecular correlated electronic decay phenomena observed in superfluid helium nanodroplets subjected to extreme ultraviolet radiation. Helium nanodroplets, known for their distinctive electronic and quantum fluid properties, provide an ideal environment for examining a variety of non-local electronic decay processes involving the transfer of energy, charge, or both between neighboring sites and resulting in ionization and the emission of low-kinetic energy electrons. Key processes include interatomic or intermolecular Coulombic decay and its variants, such as electron transfer-mediated decay. Insights gained from studying these light-matter interactions in helium nanodroplets enhance our understanding of the effects of ionizing radiation on other condensed-phase systems, including biological matter. We also emphasize the advanced experimental and computational techniques that make it possible to resolve electronic decay processes with high spectral and temporal precision. Utilizing ultrashort pulses from free-electron lasers, the temporal evolution of these processes can be followed, significantly advancing our comprehension of the dynamics within quantum fluid clusters and non-local electronic interactions in nanoscale systems.
Keyword:
Helium nanodroplets
interatomic coulombic decay
photoionization
quantum fluid
synchrotron spectroscopy
free-electron lasers

期刊

Reports on Progress in Physics 封面图
Reports on Progress in Physics
IF:
20.7
论文数:
1.6K
被引数:
2.4W

机构

A
Aarhus University
学者数:
4.3W
论文数: 4.2W
被引数: 4.8W
I
indian institute of technology system (iit system)
学者数:
9.5W
论文数: 9.9W
被引数: 93
U
University of Connecticut
学者数:
2.4W
论文数: 2.2W
被引数: 2.5W
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