Interfacial catalysis in enzymatic PET plastic depolymerization

Jie Zhou

doi:10.1016/j.trechm.2025.02.005

2025-04-01

PRE

DOI：10.1016/j.trechm.2025.02.005

原文链接

原文求助

摘要

En 中文

固液界面上的界面催化在众多自然和工业过程中发挥着关键作用，包括塑料废料的酶解解聚。在适用于生物基聚酯的各种聚酯水解酶的发现和工程化方面已取得显著进展，但对由生物催化解聚引起的聚合物表面侵蚀过程的表征仍处于早期阶段。在此，我们旨在理解聚合物与酶之间的界面特性，以及它们的相互作用、反应动力学和传质过程如何影响酶解解聚的速率和程度。我们预期，弥合蛋白质工程与过程工程之间的差距将开辟出工程化更优生物催化剂并加速塑料废料生物处理的途径。

Keyword:

DEGRADATION

HYDROLYSIS

IMPACT

FILMS

期刊

Trends in Chemistry

IF:

13.6

论文数:

827

被引数:

5.7K

机构

暂无机构信息

引用论文

From Bulk to Binding: Decoding the Entry of PET into Hydrolase Binding Pockets

JACS AU

IF8.7

2024-09-26

OAAI

Jaeckering, Anna; Goettsch, Frederike; Scha''ffler, Moritz; Doerr, Mark; Bornscheuer, Uwe T.; Wei, Ren; Strodel, Birgit

Rapid depolymerization of poly(ethylene terephthalate) thin films by a dual-enzyme system and its impact on material properties

CHEM CATALYSIS

IF11.6

2022-12-01

OAAI

Tarazona, Natalia A.; Wei, Ren; Brott, Stefan; Pfaff, Lara; Bornscheuer, Uwe T.; Lendlein, Andreas; Machatschek, Rainhard

Temporal and spatial evolution of enzymatic degradation of amorphous PET plastics

NPJ MATERIALS DEGRADATION

IF7.6

2022-11-12

OAAI

Lippold, Holger; Kahle, Laura; Sonnendecker, Christian; Matysik, Joerg; Fischer, Cornelius

Degradation Rates of Plastics in the Environment 塑料在环境中的降解率

ACS SUSTAINABLE CHEMISTRY & ENGINEERING

IF7.3

2020-02-03

1.9K

OAAI

Chamas, Ali; Moon, Hyunjin; Zheng, Jiajia; Qiu, Yang; Tabassum, Tarnuma; Jang, Jun Hee; Abu-Omar, Mandi; Scott, Susannah L.; Suh, Sangwon

UV Pretreatment Impairs the Enzymatic Degradation of Polyethylene Terephthalate

FRONTIERS IN MICROBIOLOGY

IF4.5

2020-04-28

OAAI

Falkenstein, Patricia; Graesing, Daniel; Bielytskyi, Pavlo; Zimmermann, Wolfgang; Matysik, Joerg; Wei, Ren; Song, Chen

Natural depolymerization of waste poly(ethylene terephthalate) by neutral hydrolysis in marine water

SCIENTIFIC REPORTS

IF3.9

2021-02-24

OAAI

Stanica-Ezeanu, Dorin; Matei, Danuta

Merging Plastics, Microbes, and Enzymes: Highlights from an International Workshop

APPLIED AND ENVIRONMENTAL MICROBIOLOGY

IF3.7

2022-07-26

OAAI

Jimenez, Diego Javier; Oezturk, Basak; Wei, Ren; Bugg, Timothy D.; Amaya Gomez, Carol Viviana; Salcedo Galan, Felipe; Castro-Mayorga, Jinneth Lorena; Saldarriaga, Juan Fernando; Tarazona, Natalia Andrea

Deep learning guided enzyme engineering of Thermobifida fusca cutinase for increased PET depolymerization

Chinese Journal of Catalysis

IF17.7

2023-07-01

OAAI

Meng, Shuaiqi; Li, Zhongyu; Zhang, Peng; Contreras, Francisca; Ji, Yu; Schwaneberg, Ulrich

Bridging the Gap in the Structure–Function Paradigm of Enzymatic PET Degradation–Aromatic Residue Driven Balanced Interactions with Catalytic and Anchoring Subsite 填补酶促PET降解结构-功能范式中的差距——芳香族残基驱动的催化亚位和锚定亚位之间的平衡相互作用

ChemBioChem

IF0

2024-10-17

PREAI

Anjima James; Anjitha Bhasi; Susmita De