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Machine-learning-assisted insight into spin ice Dy2Ti2O7
DOI:10.1038/s41467-020-14660-y.png)
摘要
En 中文
Complex behavior poses challenges in extracting models from experiment. An example is spin liquid formation in frustrated magnets like Dy2Ti2O7. Understanding has been hindered by issues including disorder, glass formation, and interpretation of scattering data. Here, we use an automated capability to extract model Hamiltonians from data, and to identify different magnetic regimes. This involves training an autoencoder to learn a compressed representation of three-dimensional diffuse scattering, over a wide range of spin Hamiltonians. The autoencoder finds optimal matches according to scattering and heat capacity data and provides confidence intervals. Validation tests indicate that our optimal Hamiltonian accurately predicts temperature and field dependence of both magnetic structure and magnetization, as well as glass formation and irreversibility in Dy2Ti2O7. The autoencoder can also categorize different magnetic behaviors and eliminate background noise and artifacts in raw data. Our methodology is readily applicable to other materials and types of scattering problems.
Keyword:
COULOMB PHASE
STATE
OPTIMIZATION
AI总结
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期刊
IF:
15.7
论文数:
9.3W
被引数:
91.2W
机构
引用论文
Intermediate magnetization state and competing orders in Dy2Ti2O7 and Ho2Ti2O7
NATURE COMMUNICATIONS
IF15.7

