.png){kind=icon}
返回
Mapping and Modeling Physicochemical Fields in Solid-State Batteries
.png){kind=icon}
PRE
AI
DOI：10.1021/acs.jpclett.2c02800.png)
.png){kind=icon}
原文求助.png){kind=icon}
分享.png){kind=icon}
收藏
摘要
En 中文
The safety and energy density of solid-state batteries can be, in principle, substantially increased compared with that of conventional lithium-ion batteries. However, the use of solid-state electrolytes instead of liquid electrolytes introduces pronounced complexities to the solid-state system because of the strong coupling between different physicochemical fields. Understanding the evolution of these fields is critical to unlocking the potential of solid-state batteries. This necessitates the development of experimental and theoretical methods to track electrochemical, stress, crack, and thermal fields upon battery cycling. In this Perspective, we survey existing characterization techniques and the current understanding of multiphysics coupling in solid-state batteries. We propose that the development of experimental tools that can map multiple fields concurrently and systematic consideration of material plasticity in theoretical modeling are important for the advancement of this emerging battery technology. This Perspective provides introductory material on solid-state batteries to scientists from a broad physical chemistry community, motivating innovative and interdisciplinary studies in the future.
Keyword:
IONIC-CONDUCTIVITY
LITHIUM
ELECTROLYTES
DEFORMATION
ORIGIN
PROPAGATION
STABILITY
FRACTURE
期刊
IF:
4.6
论文数:
2.6K
被引数:
7.4W
机构
引用论文
Fast lithium growth and short circuit induced by localized-temperature hotspots in lithium batteries锂电池局部温度热点引起的锂快速生长和短路.png)
NATURE COMMUNICATIONS
OAAI
NATURE COMMUNICATIONSIF15.7
OAAI分享收藏Coupled crack propagation and dendrite growth in solid electrolyte of all-solid-state battery全固态电池固体电解质中裂纹扩展和枝晶生长的耦合NANO ENERGYOAAI
NANO ENERGYIF17.1
OAAI分享收藏Impedance-Based Battery Management System for Safety Monitoring of Lithium-Ion Batteries基于阻抗的锂离子电池安全监测电池管理系统
PREAI
分享收藏分享收藏High-throughput production of force-fields for solid-state electrolyte materials固态电解质材料力场的高通量生产APL MATERIALSOAAI
APL MATERIALSIF4.5
OAAI分享收藏Lithium ionic conductor thio-LISICON -: The Li2S-GeS2-P2S5 system锂离子导体thio-lisicon-: Li2S-GeS2-P2S5系统
PREAI
分享收藏
查看更多内容