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Multielectron Dynamics in the Condensed Phase: Quantum Structure-Function Relationships
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DOI：10.1146/annurev-physchem-042018-052515.png)
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摘要
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Quantum information promises dramatic advances in computing last seen in the digital revolution, but quantum hardware is fragile, noisy, and resource intensive. Chemistry has a role in developing new materials for quantum information that are robust to noise, scalable, and operable in ambient conditions. While molecular structure is the foundation for understanding mechanism and reactivity, molecular structure/quantum function relationships remain mostly undiscovered. Using singlet fission as a specific example of a multielectron process capable of producing long-lived spin-entangled electronic states at high temperatures, I describe how to exploit molecular structure and symmetry to gain quantum function and how some principles learned from singlet fission apply more broadly to quantum science.
Keyword:
spin polarization
quantum computing
singlet fission
electron paramagnetic resonance
quantum dynamics
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