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Non-reciprocal linearly polarized light in simple media

delete2026-07-27
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PRE
AI
T
Thomas J. Ugras
D
Daniel J. Gracias
R
Reilly P. Lynch
O
Oriol Arteaga
R
Richard D. Robinson *
DOI:10.1038/s41563-026-02660-0delete
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Abstract

Abstract

En 中文
Reciprocity—the principle that a response is identical along the forward and backward paths—is a fundamental concept across physics. Non-reciprocity occurs when this symmetry is broken, resulting in direction-dependent behaviour. Achieving optical non-reciprocity typically requires complex metamaterials, exotic media or strong fields. Researchers have overlooked the possibility that conventional materials could support optical non-reciprocity. Here, through the Stokes–Mueller formalism, we predict a pathway to non-reciprocal absorption and emission of orthogonal linear polarizations. We test this idea using solution-processed films of CdS, CdSe and CdTe magic-size clusters with comparable circular and linear dichroism, and demonstrate non-reciprocal absorption and emission of linearly polarized light. Based on these findings, several design rules and practical applications are presented. Our work reveals that non-reciprocal linear dichroism and emission can be achieved in readily processable materials by harnessing chiral–linear optical interference, providing opportunities within polarization-based quantum optics and photonics such as direction-dependent optical routing or polarization-multiplexed encryption. Directional asymmetry in light absorption and emission emerges in simple materials from the interplay of chirality and linear anisotropy.

Journal

Nature Materials cover
Nature Materials
IF:
38.5
Papers:
6.7K
Citations:
11.5W

Organization

U
universitat de barcelona
Scholars:
1.2K
Papers: 501
Citations: 0
C
cornell university
Scholars:
4.1K
Papers: 1.7K
Citations: 0
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