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Nonlinear mid-infrared meta-membranes

delete2024-07-24
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OA
AI
G
Giovanni Sartorello
J
Joshua Bocanegra
D
David Knez
D
Daniil M. Lukin
J
Joshua Yang
J
Jelena Vučković
D
Dmitry A. Fishman
G
Gennady Shvets
M
Maxim R. Shcherbakov *
DOI:10.1515/nanoph-2024-0203delete
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Abstract

Abstract

En 中文
Nanophotonic structures have shown promising routes to controlling and enhancing nonlinear optical processes at the nanoscale. However, most nonlinear nanostructures require a handling substrate, reducing their application scope. Due to the underwhelming heat dissipation, it has been a challenge to evaluate the nonlinear optical properties of free-standing nanostructures. Here, we overcome this challenge by performing shot-controlled fifth harmonic generation (FHG) measurements on a SiC meta-membrane - a free-standing transmission metasurface with pronounced optical resonances in the mid-infrared (lambda res approximate to 4,000 nm). Back focal plane imaging of the FHG diffraction orders and rigorous finite-difference time-domain simulations reveal at least two orders of magnitude enhancement of the FHG from the meta-membrane, compared to the unstructured SiC film of the same thickness. Single-shot measurements of the meta-membrane with varying resonance positions reveal an unusual spectral behavior that we explain with Kerr-driven intensity-dependent resonance dynamics. This work paves the way for novel substrate-less nanophotonic architectures.
Keywords:
metasurfaces
nonlinear optics
silicon carbide
mid-infrared
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Nanophotonics cover
Nanophotonics
IF:
6.6
Papers:
2.9K
Citations:
1.6W

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University of California System cover
University of California System
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Cornell University
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university of california irvine
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