.png){kind=icon}
返回
Oxide-Based Solid-State Batteries: A Perspective on Composite Cathode Architecture
.png){kind=icon}
OA
AI
DOI：10.1002/aenm.202201939.png)
.png){kind=icon}
.png){kind=icon}
分享.png){kind=icon}
收藏
摘要
En 中文
The garnet-type phase Li7La3Zr2O12 (LLZO) attracts significant attention as an oxide solid electrolyte to enable safe and robust solid-state batteries (SSBs) with potentially high energy density. However, while significant progress has been made in demonstrating compatibility with Li metal, integrating LLZO into composite cathodes remains a challenge. The current perspective focuses on the critical issues that need to be addressed to achieve the ultimate goal of an all-solid-state LLZO-based battery that delivers safety, durability, and pack-level performance characteristics that are unobtainable with state-of-the-art Li-ion batteries. This perspective complements existing reviews of solid/solid interfaces with more emphasis on understanding numerous homo- and heteroionic interfaces in a pure oxide-based SSB and the various phenomena that accompany the evolution of the chemical, electrochemical, structural, morphological, and mechanical properties of those interfaces during processing and operation. Finally, the insights gained from a comprehensive literature survey of LLZO-cathode interfaces are used to guide efforts for the development of LLZO-based SSBs.
Keyword:
ceramic cathode
electrolyte interface
grain boundaries
oxide solid electrolyte
solid state battery
AI总结
对已上传原文的论文进行重点信息的提取，主要内容包括：简要概述、研究摘要、背景介绍、关键亮点、图文解析、展望与总结。
期刊
IF:
26
论文数:
1.0W
被引数:
15.7W
机构
引用论文
3D lithium metal anodes hosted in asymmetric garnet frameworks toward high energy density batteries在不对称石榴石框架中承载的3D锂金属阳极用于高能量密度电池.png)
ENERGY STORAGE MATERIALSOAAI
ENERGY STORAGE MATERIALSIF20.2
OAAI分享收藏分享收藏Problem, Status, and Possible Solutions for Lithium Metal Anode of Rechargeable Batteries可充电电池锂金属阳极的问题、现状和可能的解决方案
PREAI
分享收藏Resolving the Discrepancy in Tortuosity Factor Estimation for Li-Ion Battery Electrodes through Micro-Macro Modeling and Experiment通过微宏建模和实验解决锂离子电池电极曲折因子估计的差异
OAAI
OAAI分享收藏Ga-substituted Li7La3Zr2O12: An investigation based on grain coarsening in garnet-type lithium ion conductorsGa取代的Li7La3Zr2O12: 基于石榴石型锂离子导体中晶粒粗化的研究
PREAI
分享收藏First-Principles Modeling of Mn(II) Migration above and Dissolution from LixMn2O4 (001) SurfacesMn(II) 在LixMn2O4 (001) 表面上方迁移和溶解的第一性原理模型OAAI
OAAI分享收藏Mechanical and Electrochemical Response of a LiCoO2 Cathode using Reconstructed Microstructures使用重建的微观结构的LiCoO2阴极的机械和电化学响应ELECTROCHIMICA ACTAOAAI
ELECTROCHIMICA ACTAIF5.6
OAAI分享收藏The role of Al and Li concentration on the formation of cubic garnet solid electrolyte of nominal composition Li7La3Zr2O12Al和Li浓度对标称组成Li7La3Zr2O12的立方石榴石固体电解质形成的作用SOLID STATE IONICS
SOLID STATE IONICSIF3.3
PREAI
分享收藏Fundamentals of inorganic solid-state electrolytes for batteries电池用无机固态电解质基础NATURE MATERIALS
NATURE MATERIALSIF38.5
PREAI
分享收藏
查看更多内容