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Process-oriented approach towards catalyst design and optimisation
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DOI：10.1016/j.catcom.2021.106392.png)
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摘要
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Translation of catalysts developed in academia to industrial end-users remains a challenge due to a lack of knowledge about the impact of catalyst attributes on the whole process and vice versa. A systematic methodology is proposed that assesses these in terms of Key Performance Indicators (KPIs). As a case study, the dehydration of butanol to butenes and dibutyl ether is considered over H-ZSM5 and H-Beta catalysts. It is demonstrated that catalysts should be designed for complete conversion and high butene selectivity, as removal of unreacted 1-butanol requires a complex separation due to the thermo-physical properties of the product mixture.
Keyword:
Catalysis
Optimisation
Process synthesis
Conceptual design
Kinetics estimation
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4.3
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6.6K
被引数:
1.3W
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Dehydration of butanol to butene over solid acid catalysts in high water environments高水环境下固体酸催化剂上丁醇脱水制丁烯.png)
JOURNAL OF CATALYSIS
JOURNAL OF CATALYSISIF6.5
PREAI
分享收藏分享收藏Reaction path analysis for 1-butanol dehydration in H-ZSM-5 zeolite: Ab initio and microkinetic modelingH-ZSM-5沸石中1-丁醇脱水的反应路径分析: 从头算和微观动力学模型JOURNAL OF CATALYSIS
JOURNAL OF CATALYSISIF6.5
PREAI
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