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Quasi-solid electrolytes using a single-cation ionic liquid
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DOI：10.1039/D5CP04903B.png)
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Abstract
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Proof-of-concept quasi-solid electrolytes (QSEs) combining Li1+x+yAlxTi2−xSiyP3−yO12 and a single-cation ionic liquid (SCIL) composed of lithium bis(fluorosulfonyl)amide and lithium (fluorosulfonyl)(trifluoromethanesulfonyl)amide are demonstrated without inducing concentration gradients. The QSEs exhibited ionic conductivities comparable to the SCIL without high-temperature sintering. These results demonstrate the potential of SCIL-based QSEs as model systems for investigating Li+ transport under concentration-gradient-free conditions in solid-state battery systems.
Keywords:
Quasi-solid electrolytes
Single-cation ionic liquid
Lithium transport
Concentration-gradient-free
Solid-state batteries
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