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Reactive nitrogen species regulating sulfadiazine degradation by biochar-activated periodate with ammonium
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DOI：10.1016/j.apcatb.2025.125979.png)
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Abstract
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• NH4+ boosted sulfadiazine degradation in biochar-activated periodate (BC/PI) systems. • •IO3 was revealed as the dominant reactive species in BC/PI. • NO2• drove accelerated sulfadiazine degradation in BC/PI/NH4+. • Energy barrier reduction for NO2• oxidation was confirmed through DFT calculations. • Nitro-byproducts with enhanced toxicity were detected in BC/PI/NH4+.
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