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Removal of trace gases can both increase and decrease cloud droplet formation

delete2026-01-14
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PRE
AI
E
Elavarasi Ravichandran
S
Sanghee Han
A
A. Williams
V
Veronica Z. Berta
J
Jeremy L. Dedrick
C
Christian Pelayo
N
Nattamon Maneenoi
L
Lynn M. Russell
M
Michael Wheeler
J
Jeremy J. B. Wentzell
J
J. Liggio
M
Markus D. Petters *
DOI:10.1126/sciadv.adx0960delete
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摘要

摘要

En 中文
气溶胶由分散在气体中的液体或固体颗粒组成。气溶胶测量通常需要在量化其物理化学性质前对颗粒进行干燥处理。这种干燥过程可能会从颗粒中去除半挥发性化合物。本研究通过尺寸分辨的云凝结核(CCN)测量,量化了有无去除装置(denuder)情况下的吸湿性参数。去除装置有效移除了气相中碳原子数少于10的烷烃以及弱功能化的酸、醛和醇。去除有机化合物使基于CCN的吸湿性参数扰动高达50%。去除过程或使颗粒的CCN活性增强或减弱,其影响方向取决于样品相对湿度和痕量气体浓度。该效应在初春最弱,在晚春和夏季最强。测量结果表明,颗粒相和气相之间存在异常强烈的耦合,通过挥发性或表面吸附,或两者共同作用,影响着CCN活性。
Keyword:
CONDENSATION NUCLEI ACTIVITY
SECONDARY ORGANIC AEROSOL
BIOMASS BURNING AEROSOL
ULTRAVIOLET ION-SOURCE
AIR-WATER-INTERFACE
CCN ACTIVITY
CRITICAL SUPERSATURATION
CHEMICAL-COMPOSITION
HYGROSCOPIC GROWTH
ATMOSPHERIC GASES

期刊

Science Advances 封面图
Science Advances
IF:
12.5
论文数:
2.1W
被引数:
20.0W

机构

U
University of California Riverside
学者数:
133
论文数: 70
被引数: 1
University of California System 封面图
University of California System
学者数:
37.7W
论文数: 33.8W
被引数: 16.0W
引用论文

引用论文

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