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Research Advances of Zeolite-Anchored Single-Atom Site Catalysts: From Rational Design to Potential Applications
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PRE
AI
Q
J
S
H
Z
王
S
DOI：10.1002/cctc.70905.png)
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Abstract
En 中文
Zeolite-supported single-atom catalysts (SACs) have displayed great potential for applications in green catalysis and energy conversion. Precisely regulating the geometric and electronic configuration and revealing the structure-activity relationships of single-atoms (SAs) inside or outside zeolites present numerous challenges. This review comprehensively summarizes the recent advances in microenvironment engineering of zeolite-anchored single-atom active sites (SAAS) in terms of design principles, synthetic methods, characterization techniques and theoretical perspectives of structure-activity relationship. Besides, the latest research progress in several typical energy catalysis processes is systematically and comprehensively explored to provide a comprehensive understanding of the catalytic mechanisms over zeolite-supported SACs. In addition, the applications of zeolites in industrial catalytic processes are in industrial catalytic processes are summarized. Finally, the challenges and potential opportunities of zeolite-based-SACs in green catalysis and energy conversion are presented. This work will offer valuable information for the advancement of zeolite-based catalysts at the atomic scale for catalytic applications.
Keywords:
green catalysis and energy conversion
microenvironment engineering
single-atom catalysts
structure-activity relationships
zeolites
Journal
IF:
3.9
Papers:
9.4K
Citations:
2.5W
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Cited Papers