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Single-amine strategy for CO2 hydrogenation to formic acid: Process simplification using NBIM coupled with heterogeneous Ru-MACHO-POMP catalysis
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DOI：10.1016/j.jcou.2026.103426.png)
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Abstract
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• Single-amine NBIM integrates CO₂ hydrogenation and formic acid separation. • Using Ru-MACHO-POMP, AAR-guided optimization defined a practical reaction–separation window. • A single-amine approach removes the need for an amine-exchange step in CO₂-to-formic acid production. • The integrated assessment confirms the feasibility of a single-amine route toward economically viable and sustainable formic acid production.
Keywords:
CO2 hydrogenation
Formic acid production
Single-amine system
Heterogeneous catalysis
TEA-LCA analysis
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