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Single-layer ionic conduction on carboxyl-terminated silane monolayers patterned by constructive lithography
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DOI：10.1038/NMAT4254.png)
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摘要
En 中文
Ionic transport plays a central role in key technologies relevant to energy, and information processing and storage, as well as in the implementation of biological functions in living organisms. Here, we introduce a supramolecular strategy based on the non-destructive chemical patterning of a highly ordered self-assembled monolayer that allows the reproducible fabrication of ion-conducting surface patterns (ion-conducting channels) with top -COOH functional groups precisely definable over the full range of length scales from nanometre to centimetre. The transport of a single layer of selected metal ions and the electrochemical processes related to their motion may thus be confined to predefined surface paths. As a generic solid ionic conductor that can accommodate different mobile ions in the absence of any added electrolyte, these ion-conducting channels exhibit bias-induced competitive transport of different ionic species. This approach offers unprecedented opportunities for the realization of designed ion-conducting systems with nanoscale control, beyond the inherent limitations posed by available ionic materials.
Keyword:
CRYSTALLINE POLYMER ELECTROLYTES
SELF-ASSEMBLED MONOLAYERS
METAL
TRANSPORT
SILVER
NANOLITHOGRAPHY
NANOPATTERNS
REPLICATION
TEMPLATES
INSIGHTS
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38.5
论文数:
6.8K
被引数:
11.5W
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