Single-spin stochastic optical reconstruction microscopy

Matthias Pfender

doi:10.1073/pnas.1404907111

2014-09-29

DOI：10.1073/pnas.1404907111

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摘要

En 中文

We experimentally demonstrate precision addressing of single-quantum emitters by combined optical microscopy and spin resonance techniques. To this end, we use nitrogen vacancy (NV) color centers in diamond confined within a few ten nanometers as individually resolvable quantum systems. By developing a stochastic optical reconstruction microscopy (STORM) technique for NV centers, we are able to simultaneously perform sub-diffraction-limit imaging and optically detected spin resonance (ODMR) measurements on NV spins. This allows the assignment of spin resonance spectra to individual NV center locations with nanometer-scale resolution and thus further improves spatial discrimination. For example, we resolved formerly indistinguishable emitters by their spectra. Furthermore, ODMR spectra contain metrology information allowing for sub-diffraction-limit sensing of, for instance, magnetic or electric fields with inherently parallel data acquisition. As an example, we have detected nuclear spins with nanometer-scale precision. Finally, we give prospects of how this technique can evolve into a fully parallel quantum sensor for nanometer resolution imaging of delocalized quantum correlations.

Keyword:

superresolution microscopy

single-spin detection

diamond defect center

nitrogen-vacancy center

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期刊

Proceedings of the National Academy of Sciences of the United States of America

IF:

9.1

论文数:

10.8W

被引数:

73.5W

机构

university of stuttgart

学者数:

275

论文数: 114

被引数: 0

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