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In the March issue of Joule, Chunsheng Wang, Xiangxin Guo, and collaborators develop a process to form an all-ceramic cathode-electrolyte composite with extremely low interfacial resistance, demonstrating excellent cycling performance in a full solid-state cell with Li metal anode, garnet-type Li7La3Zr2O12 (LLZO) electrolyte, and LiCoO2 (LCO) cathode. By taking advantage of the native Li2CO3 impurity formed on the electrolyte and cathode materials when exposed in ambient conditions, the authors outline a practical process to produce an electrochemically stable and ionically conductive interphase that wets both LLZO and LCO.
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