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Treating random sequential addition via the replica method

delete2022-08-25
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OA
AI
R
Ryan B. Jadrich *
B
Beth A. Lindquist
T
Thomas M. Truskett
DOI:10.1063/5.0096276delete
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摘要

摘要

En 中文
While many physical processes are non-equilibrium in nature, the theory and modeling of such phenomena lag behind theoretical treatments of equilibrium systems. The diversity of powerful theoretical tools available to describe equilibrium systems has inspired strategies that map non-equilibrium systems onto equivalent equilibrium analogs so that interrogation with standard statistical mechanical approaches is possible. In this work, we revisit the mapping from the non-equilibrium random sequential addition process onto an equilibrium multi-component mixture via the replica method, allowing for theoretical predictions of non-equilibrium structural quantities. We validate the above approach by comparing the theoretical predictions to numerical simulations of random sequential addition. (c) 2022 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution (CC BY) license (http://creativecommons.org/licenses/by/4.0/).

期刊

Journal of Chemical Physics 封面图
Journal of Chemical Physics
IF:
3.1
论文数:
7.2W
被引数:
23.2W

机构

U
united states department of energy (doe)
学者数:
11.3W
论文数: 9.6W
被引数: 246
L
Los Alamos National Laboratory
学者数:
9.6K
论文数: 6.7K
被引数: 1.9W
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