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Two-Dimensional Conductive π-d Frameworks with Multiple Sensory Capabilities
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DOI：10.1021/acsami.1c06596.png)
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Two-dimensional (2D) metal-molecule hybrid frameworks have attracted great attention due to their pi-d interactions for the charge-spin-lattice coupling, promising for next-generation molecular electronics. However, a high electrical conductivity is indispensable to realize such potential. Herein, we design and assemble a conductive 2D conjugated coordination thin film through an interfacial reaction between the aqueous and organic phases. Its electronic conducting properties are derived from the pi-d coupling interactions to achieve an electrical conductivity of 1.05 S/cm, while the stimulus-dependent pi-d interactions induce multifunctional sensory capabilities. The Co-DABDT (DABDT = 2,5-diamino-1,4-benzenedithiol dihydrochloride) thin films demonstrate an excellent performance for sensing light, strain, temperature, and humidity, as well as robust mechanical stability. The 2D frameworks with multisensing properties for real-time static and dynamic monitoring are promising for smart wearable electronic systems.
Keyword:
2D conductive polymers
metal-organic frameworks
self-assembly
multiple sensory capabilities
robustness
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8.2
论文数:
6.1W
被引数:
38.7W
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