arrow
返回

Visualizing nanoparticle surface dynamics and instabilities enabled by deep denoising

delete2025-02-28
delete1
PRE
AI
P
Peter A. Crozier *
M
Matan Leibovich
P
Piyush Haluai
M
Mai Tan
A
Andrew M. Thomas
J
Joshua Vincent
S
Sreyas Mohan
A
Adrià Marcos Morales
K
Kulkarni, Shreyas A.
D
David S. Matteson
Y
Yifan Wang
C
Carlos Fernandez‐Granda *
DOI:10.1126/science.ads2688delete
delete原文链接
delete原文求助
delete分享
delete收藏
摘要

摘要

En 中文
材料的功能可能与发生在毫秒时间尺度的原子级结构动力学相关。然而,电子显微镜在以高空间分辨率和毫秒时间分辨率成像结构方面的能力,通常受到信噪比较低的限制。通过一种无监督的深度去噪框架,我们在气体环境中以中等电子剂量,观察到了金属纳米颗粒表面(氧化铈上的铂纳米颗粒),时间分辨率低至10毫秒。在此时间尺度上,许多纳米颗粒表面持续在有序和无序构型之间转换。应力场可以渗透至表面以下,导致缺陷形成和失稳,从而使纳米颗粒表现出易变性。将这种无监督去噪器与原位电子显微镜相结合,显著提升了时空表征能力,为探索材料中的原子级结构动力学开启了一扇新窗口。
Keyword:
IN-SITU
CARBON-MONOXIDE
DIFFUSION

期刊

Science 封面图
Science
IF:
45.8
论文数:
1.4W
被引数:
78.6W

机构

N
NYU
学者数:
1.8K
论文数: 1.1K
被引数: 390
U
Univ Iowa
学者数:
1.2K
论文数: 951
被引数: 145
引用论文

引用论文

Imaging of Transient Structures Using Nanosecond in Situ TEM
err2008-09-12
err0
PREAI
errJudy S. Kim; Thomas LaGrange; Bryan W. Reed; Mitra L. Taheri; Michael R. Armstrong; Wayne E. King; Nigel D. Browning; Geoffrey H. Campbell
err分享
err收藏
Modified Winterbottom Construction Including Boundaries
err2020-12-09
err11
errOAAI
errMansley, Zachary R.; Marks, Laurence D.
err分享
err收藏
Topological Data Analysis with Applications
err
IF0
err2021-11-25
err0
errOAAI
errGunnar Carlsson; Mikael Vejdemo-Johansson
err分享
err收藏
Characterisation of the Idiotypic Immune Network Through Persistent Entropy
err2016-05-04
err0
PREAI
errMatteo Rucco; Filippo Castiglione; Emanuela Merelli; Marco Pettini
err分享
err收藏
Dynamic behavior of metal nanoparticles for catalysis金属纳米颗粒催化动力学行为研究
err2018-06-01
err107
PREAI
errZhou, Yan; Jin, Chuanchuan; Li, Yong; Shen, Wenjie
err分享
err收藏
Atomic-Scale Mechanism of Platinum Catalyst Restructuring under a Pressure of Reactant Gas
err2022-12-22
err16
PREAI
errSumaria, Vaidish; Nguyen, Luan; Tao, Franklin Feng; Sautet, Philippe
err分享
err收藏
Deep Denoising for Scientific Discovery: A Case Study in Electron Microscopy
err2022-01-01
err0
errOAAI
errSreyas Mohan; Ramon Manzorro; Joshua L. Vincent; Binh Tang; Dev Y. Sheth; Eero P. Simoncelli; David S. Matteson; Peter A. Crozier; Carlos Fernandez-Granda
err分享
err收藏
学者 查看更多内容