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Anomalously High Activity in a Nonporous Catalyst: Oxidative Desulfurization Enabled by an Ultralow Surface Area Amorphous Co(II)–BDC Coordination Polymer
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DOI：10.1016/j.apcatb.2026.126908.png)
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Abstract
En 中文
• An amorphous Co(II)-BDC coordination polymer with ultralow surface area is synthesized. • It exhibits superior catalytic activity in PMS-activated oxidative desulfurization. • Strong PMS chemisorption and electronic modulation of Co-centers contribute to the exceptional activity. • Kinetic analysis reveals a consecutive reaction pathway with a rate-determining deep oxidation step.
Keywords:
Co(II)-BDC coordination polymer
oxidative desulfurization
peroxymonosulfate activation
catalytic activity
electronic modulation
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