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Catalyst coating effects on CO2 methanation kinetics in structured reactors
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DOI：10.1016/j.jcou.2026.103449.png)
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Abstract
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• Catalyst coating method influences kinetic parameters in CO₂ methanation. • Low‑ and high‑viscosity slurry coatings yield distinct Ni reactivation behavior. • Optimal calcination temperatures prevent Ni reoxidation while removing organics • Spatially resolved data enable robust estimation of Langmuir–Hinshelwood kinetics. • Kinetic model validated in a multilayer catalytic plate reactor.
Keywords:
CO2 methanation
Catalyst coating
Kinetic study
Power-to-Gas
Catalytic plate reactor
Catalytic heat exchanger
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