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Catalytic hydrogenolysis of lignin over Ni/CeO2-Al2O3 catalysts with formic acid as hydrogen source
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DOI：10.1016/j.catcom.2024.106868.png)
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Abstract
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Lignin is an aromatic polymer with prospects for producing high value-added chemicals. In this study, hydrogenolysis of alkaline lignin was carried out at 240 degrees C for 8 h in a hydrothermal kettle using Ni/xCeO2-yAl2O3 as catalyst and formic acid as hydrogen source. Compared with Ni catalysts supported by single oxides, the results showed that Ni/xCeO2-yAl2O3 composite-supported catalysts exhibited better catalytic depolymerization performance with higher bio-oil yields. Among them, Ni/1CeO2-3Al2O3 exhibited the most outstanding catalytic activity, with a bio-oil yield of 52.77 wt% and a phenolic compound yield of 7.21 wt%.
Keywords:
Biomass
Lignin
Bio-oil
Metallic oxide
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