arrow
Return

Challenges in speeding up solid-state battery development

delete2023-02-23
delete449
PRE
AI
J
Jürgen Janek *
W
Wolfgang G. Zeier *
DOI:10.1038/s41560-023-01208-9delete
deleteOriginal
deleteOriginal request for help
deleteShare
deleteSave
Abstract

Abstract

En 中文
Recent worldwide efforts to establish solid-state batteries as a potentially safe and stable high-energy and high-rate electrochemical storage technology still face issues with long-term performance, specific power and economic viability. Here, we review key challenges that still involve the need for fast-conducting solid electrolytes to provide sufficient transport in composite cathodes. In addition, we show that high-performance anodes together with protection concepts are paramount to establish dense high-energy solid-state batteries and that lithium-based solid-state batteries as well as metal anodes may not be the ultimate solution. We further discuss that diversity in terms of materials, research teams and approaches is key to establish long-term solid-state batteries. About ten years after the first ground-breaking publication of lithium solid electrolytes with an ionic conductivity higher than that of liquid electrolytes, it is time to realistically address the remaining key challenges for full-scale commercialization, cell performance and implementation. Solid-state batteries are widely regarded as one of the next promising energy storage technologies. Here, Wolfgang Zeier and Juergen Janek review recent research directions and advances in the development of solid-state batteries and discuss ways to tackle the remaining challenges for commercialization.
Keywords:
LITHIUM-ION CONDUCTIVITY
SUPERIONIC CONDUCTORS
ELECTROCHEMICAL PROPERTIES
CRYSTAL-STRUCTURE
ELECTROLYTES
LI
DYNAMICS
ANODES
LI7LA3ZR2O12
LI10GEP2S12

Journal

Nature Energy cover
Nature Energy
IF:
60.1
Papers:
1.0K
Citations:
5.6W

Organization

K
karlsruhe institute of technology
Scholars:
2.0W
Papers: 1.5W
Citations: 23
J
justus liebig university giessen
Scholars:
1.5W
Papers: 1.2W
Citations: 95
Cited Papers

Cited Papers

Grafted polyrotaxanes as highly conductive electrolytes for lithium metal batteries
err2019-01-01
err72
PREAI
errImholt, Laura; Doerr, Tobias S.; Zhang, Peng; Ibing, Lukas; Cekic-Laskovic, Isidora; Winter, Martin; Brunklaus, Gunther
errShare
errSave
Post-lithium-ion battery cell production and its compatibility with lithium-ion cell production infrastructure
err2021-01-28
err785
PREAI
errDuffner, Fabian; Kronemeyer, Niklas; Tuebke, Jens; Leker, Jens; Winter, Martin; Schmuch, Richard
errShare
errSave
High-energy long-cycling all-solid-state lithium metal batteries enabled by silver-carbon composite anodes
err2020-03-09
err1.1K
PREAI
errLee, Yong-Gun; Fujiki, Satoshi; Jung, Changhoon; Suzuki, Naoki; Yashiro, Nobuyoshi; Omoda, Ryo; Ko, Dong-Su; Shiratsuchi, Tomoyuki; Sugimoto, Toshinori; Ryu, Saebom; Ku, Jun Hwan; Watanabe, Taku; Park, Youngsin; Aihara, Yuichi; Im, Dongmin; Han, In Taek
errShare
errSave
Local electronic structure variation resulting in Li 'filament' formation within solid electrolytes
err2021-05-31
err298
PREAI
errLiu, Xiaoming; Garcia-Mendez, Regina; Lupini, Andrew R.; Cheng, Yongqiang; Hood, Zachary D.; Han, Fudong; Sharafi, Asma; Idrobo, Juan Carlos; Dudney, Nancy J.; Wang, Chunsheng; Ma, Cheng; Sakamoto, Jeff; Chi, Miaofang
errShare
errSave
errShare
errSave
Review-Practical Challenges Hindering the Development of Solid State Li Ion Batteries
err2017-06-09
err623
errOAAI
errKerman, Kian; Luntz, Alan; Viswanathan, Venkatasubramanian; Chiang, Yet-Ming; Chen, Zhebo
errShare
errSave
Inducing High Ionic Conductivity in the Lithium Superionic Argyrodites Li6+x P1-xGexS5l for All -Solid-State Batteries
err2018-11-01
err369
errOAAI
errKraft, Marvin A.; Ohno, Saneyuki; Zinkevich, Tatiana; Koerver, Raimund; Culver, Sean P.; Fuchs, Till; Senyshyn, Anatoliy; Indris, Sylvio; Morgan, Benjamin J.; Zeier, Wolfgang G.
errShare
errSave
Enhancement of ion transport in polymer electrolytes by addition of nanoscale inorganic oxides
err2001-07-01
err308
PREAI
errChung, SH; Wang, Y; Persi, L; Croce, F; Greenbaum, SG; Scrosati, B; Plichta, E
errShare
errSave
researcher View more