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Collaborative catalysis for solar biosynthesis

delete2023-02-01
delete7
PRE
AI
J
Jin‐Hyun Kim
C
Chan Beum Park *
DOI：10.1016/j.trechm.2022.11.005delete
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Abstract

Abstract

En 中文
Biocatalytic photosynthesis combines the distinctive characteristics of redox biocatalysis and photocatalysis for solar-to-chemical conversion. Photocatalytic materials harvest renewable solar light to activate oxidoreductases that offer nature-inspired routes for sustainable chemical synthesis with unparalleled reaction selectivity. Here we begin with a conceptual discussion on solarpowered redox biocatalysis, describe the underlying molecular mechanisms and thermodynamics, and highlight recent advances in: (i) photocatalytic activation of cell-free or whole-cell biocatalytic machineries (e.g., redox enzymes, acetogens, cyanobacteria); (ii) repurposing cofactor-dependent enzymes for their new-to-nature syntheses; (iii) chemical transformations by photoenzymes; and (iv) photoelectrocatalytic biosynthesis.
Keywords:
NANOWIRE-BACTERIA HYBRIDS
CARBON-DIOXIDE
CO2
LIGHT
PHOTOCATALYST
LIGNIN
OXYFUNCTIONALIZATION
BIOCATALYSIS
REDUCTION
OXIDATION

Journal

Trends in Chemistry cover
Trends in Chemistry
IF:
13.6
Papers:
813
Citations:
5.7K

Organization

No organization information available