Direct conversion of N2 and CH4 to valuable N-containing compounds via a plasma-activated catalytic process

Di Li

doi:10.1016/j.chempr.2026.103136

Direct conversion of N2 and CH4 to valuable N-containing compounds via a plasma-activated catalytic process

2026-07-10

0

PRE

AI

D

Di Li

Z

Ziming Liu

C

Chenxin Wu

T

Tao Sha

L

Li Yi

C

Chengyuan Liu

Y

Yanting Liu

L

Lei Hua

H

Haiyang Li

X

Xuhui Geng

C

Chunlei Xiao

Y

Yang Pan

L

Liang Yu *

D

Dehui Deng *

DOI：10.1016/j.chempr.2026.103136

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Abstract

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• Plasma-catalysis synergy enables direct conversion of N2 and CH4 to alkylamines and NH3 • Achieved productivities of 0.88 and 6.43 mmol gNi−1 h−1 for alkylamines and ammonia • Enhanced reaction efficiency and N–C coupling through plasma-catalytic synergy • Ni catalyst boosts conversion of excited-state N2 for N–C and N–H coupling

Direct conversion of N2 and CH4 to valuable N-containing compounds via a plasma-activated catalytic process

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