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Docking single metal sites by ion templating towards catalytic acetylene hydrochlorination
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DOI：10.1016/j.gce.2026.08.001.png)
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Abstract
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• Alkali metal ions are used as sacrificial single-ion templates to construct well-defined nitrogen-defect anchoring sites on carbon supports. • The as-prepared Au/NAC-Li catalyst exhibits outstanding activity, nearly 100% VCM selectivity, and excellent long-term stability for acetylene hydrochlorination. • The ion-templating strategy strengthens metal-support interaction, stabilizes cationic Au species, and optimizes reactant adsorption balance.
Keywords:
Acetylene hydrochlorination
Au-based catalyst
Single-ion template
Metal-support interaction
Catalytic stability
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