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Efficient yellow-green emission from Mn2+-doped (TDMP)ZnCl4 realized by the Mn-Mn ferromagnetic coupling
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DOI：10.1016/j.jlumin.2026.122022.png)
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Abstract
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• Mn2+-doped zero-dimensional (0D) (TDMP)ZnCl4 single crystals are synthesized by a solvothermal method, showing bright yellow-green emission at 550 nm. • Weak exciton magnetic polarons (EMPs) are formed at a critical Mn–Mn ferromagnetic coupling distance of ∼7.03 Å, giving a photoluminescence quantum yield (PLQY) of 99.23%. • The emission region of Mn2+ is successfully extended from green to yellow-green, providing a new approach for emission tuning of metal halides. • The fabricated light-emitting diode (LED) presents stable yellow-green emission, showing great potential in solid-state lighting.
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