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Elastomers Grow into Actuators
DOI:10.1002/adma.202209853.png)
Abstract
En 中文
It is common knowledge that when an elastomer (rubber) is stretched, its length will be maintained if its two ends are fixed. Here, it is serendipitously found that when an elastomer is slowly elongated further to achieve buckling under such conditions, the final length is much longer than the pre-stretched length. This allows the design of untethered autonomous synthetic-material-based soft robots that do not need any other chemical or electrical energy sources or external stimuli after the pre-strain is installed. Once the growth starts, the elongation continues to proceed even when the applied force is removed. Moreover, the elastomer, after growing, eventually forms a robust soft actuator that can be reshaped for different purposes. Few synthetic materials can grow like this, so far. This investigation shows that the material has an uncommon liquid crystal phase. Contrary to normal liquid crystals, it becomes birefringent only at high temperatures. The formation and the reshaping of the resulting soft actuators relate to a usually unnoticed reversible reaction. The work is promising to promote further understanding of dynamic covalent chemistry and liquid crystal elastomers, as well as to foster new designs and high-impact applications of bioinspired sustainable soft actuators in areas other than soft robots.
Keywords:
covalently adaptable networks
liquid crystal elastomers
soft actuators
soft robotics
vitrimers
Journal
IF:
26.8
Papers:
3.5W
Citations:
46.0W
Organization
Cited Papers
Locally controllable magnetic soft actuators with reprogrammable contraction-derived motions
SCIENCE ADVANCES
IF12.5
Mouldable liquid-crystalline elastomer actuators with exchangeable covalent bonds
NATURE MATERIALS
IF38.5
Internal constraints and arrested relaxation in main-chain nematic elastomers
NATURE COMMUNICATIONS
IF15.7

