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Heteroatom-doped M-N-C catalysts for oxygen reduction reactions: Doping strategies and active site regulation

delete2023-08-01
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PRE
AI
张羽 cover
张羽 (Yu Zhang)
S
Siyuan Zhu
X
Xian Wang
Z
Zhao Jin
葛君杰 (Junjie Ge)
C
Changpeng Liu
邢巍 (Wei Xing) *
DOI:10.1016/j.jelechem.2023.117506delete
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Abstract

Abstract

En 中文
M-N-C catalyst is the most potential alternative candidate for precious metal-based catalyst and has been widely concerned by researchers in recent years. As a simple and effective means, heteroatom doping is widely used to improve catalyst performance. It has been proved that heteroatom can adjust the intrinsic activity of catalyst sites by optimizing the electronic structure of MNx active sites. This review provides a comprehensive discussion on the influence of heteroatom doping on catalytic activity and the modulation of active centers in M-N-C catalysts. The various methods of introducing heteroatoms into M-N-C catalysts are thoroughly examined, and common strategies for heteroatom doping are summarized. Additionally, this article addresses current challenges in the research of M-N-C catalysts and suggests potential future directions for their development.
Keywords:
Electrocatalysis
M -N -C catalysts
Oxygen reduction reaction
Heteroatom doping

Journal

Journal of Electroanalytical Chemistry cover
Journal of Electroanalytical Chemistry
IF:
4.1
Papers:
1.7W
Citations:
4.0W

Organization

C
chinese academy of sciences
Scholars:
54.9W
Papers: 44.5W
Citations: 703
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