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Hyperbolic whispering-gallery phonon polaritons in boron nitride nanotubes

delete2023-02-23
delete16
PRE
AI
X
Xiangdong Guo
N
Ning Li
X
Xiaoxia Yang
R
Ruishi Qi
C
Chenchen Wu
R
Ruochen Shi
李跃辉 (Yuehui Li)
Y
Yang Huang
F
F. Javier Garcı́a de Abajo *
E
Enge Wang
高鹏 (Peng Gao) *
戴庆 (Qing Dai) *
DOI:10.1038/s41565-023-01324-3delete
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Abstract

Abstract

En 中文
Light confinement in nanostructures produces an enhanced light-matter interaction that enables a vast range of applications including single-photon sources, nanolasers and nanosensors. In particular, nanocavity-confined polaritons display a strongly enhanced light-matter interaction in the infrared regime. This interaction could be further boosted if polaritonic modes were moulded to form whispering-gallery modes; but scattering losses within nanocavities have so far prevented their observation. Here, we show that hexagonal BN nanotubes act as an atomically smooth nanocavity that can sustain phonon-polariton whispering-gallery modes, owing to their intrinsic hyperbolic dispersion and low scattering losses. Hyperbolic whispering-gallery phonon polaritons on BN nanotubes of similar to 4 nm radius (sidewall of six atomic layers) are characterized by an ultrasmall nanocavity mode volume (V-m approximate to 10(-10)lambda(3)(0) at an optical wavelength lambda(0) approximate to 6.4 mu m) and a Purcell factor (Q/V-m) as high as 10(12). We posit that BN nanotubes could become an important material platform for the realization of one-dimensional, ultrastrong light-matter interactions, with exciting implications for compact photonic devices.
Keywords:
FREE-ELECTRONS
NANOSPECTROSCOPY
PLASMONS
CAVITIES

Journal

Nature Nanotechnology cover
Nature Nanotechnology
IF:
34.9
Papers:
4.8K
Citations:
8.1W

Organization

B
barcelona institute of science & technology
Scholars:
1.2W
Papers: 9.7K
Citations: 36
U
university of chinese academy of sciences, cas
Scholars:
4.1W
Papers: 3.8W
Citations: 75
P
peking university
Scholars:
11.6W
Papers: 8.6W
Citations: 146
C
chinese academy of sciences
Scholars:
55.3W
Papers: 44.6W
Citations: 704
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