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In situ Bunsen reaction coupled with HI electrolysis for hydrogen production from sulfur-containing emissions
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DOI：10.1016/j.fuproc.2026.108470.png)
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Abstract
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• This work invented iodine-iodide redox loop in the anodic side of HI electrolysis to produce H2. • This invention introduces the Bunsen reaction to the anodic chamber to realize the 2I− ⇌ I2 loop. • CV/LSV confirms EC coupling mechanism and convection-dependent I2 film removal. • Sulfite-to-HI ratio governs reaction pathway, enabling process tunability. • This invention will potentially simplify the S-I cycle and H2S splitting cycle for H2 production.
Keywords:
Hydrogen production
H2S splitting cycle
S-I cycle
Bunsen reaction
HI electrolysis
Electrochemical coupling
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