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Interface engineering in LGPS-type solid-state electrolytes for all-solid-state lithium batteries

delete2024-07-01
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PRE
AI
S
Shuai Jian
H
Hongda Li *
X
Xiaobo Jia
D
Dailin Zhong
陶勃然 cover
陶勃然 (Boran Tao)
何雄 cover
何雄 (Xiong He)
G
Guofu Wang
H
Haixin Chang
DOI:10.1016/j.flatc.2024.100693delete
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Abstract

Abstract

En 中文
As key components of next-generation battery energy storage systems, solid-state batteries have attracted widespread attention. Li10GeP2S12 (LGPS)-type solid-state electrolytes (SSEs) are favored by researchers owing to their excellent ionic conductivity and potential high-temperature stability. However, the poor interface between LGPS-type SSEs and electrodes has seriously hindered the commercialization of LGPS all-solid-state lithium batteries. This review introduces the structure and Li-ion conduction mechanisms of LGPS-type SSEs and discusses the challenges related to LGPS-type SSEs/electrode interfaces, along with strategies for overcoming these challenges. To improve the interface compatibility, researchers have developed feasible methods for improving and optimizing LGPS-type SSEs. The review concludes with potential research directions and prospects of future LGPS all-solid-state lithium batteries.
Keywords:
Interface engineering
solid-state electrolytes (SSEs)
All-solid-state lithium batteries (ASSLBs)

Journal

FlatChem cover
FlatChem
IF:
6.2
Papers:
368
Citations:
2.9K

Organization

C
chinese academy of sciences
Scholars:
56.7W
Papers: 45.0W
Citations: 704
Cited Papers

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