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Interfacial catalysis in enzymatic PET plastic depolymerization

delete2025-04-01
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PRE
AI
J
Jie Zhou
崔
崔中利 (Zhongli Cui)
J
Jiang, Min
DOI:10.1016/j.trechm.2025.02.005delete
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Abstract

Abstract

En 中文
Interfacial catalysis at the solid/liquid interface plays a crucial role in numerous natural and industrial processes, including the enzymatic depolymerization of plastic waste. Significant advancements have been made in the discovery and engineering of various polyester hydrolases applicable for bio-based poly ing of the polymer surface erosion processes caused by biocatalytic depolymerization is still in its early stages. Herein, we seek to understand how the interfacial characteristics between polymers and enzymes, as well as their interaction, reaction kinetics, and mass transfer processes, influence the rate and extent of enzymatic depolymerization. We anticipate that bridging the gap between protein and process engineering will pave the way to engineer better biocatalysts and accelerate plastic waste bioprocessing.
Keywords:
DEGRADATION
HYDROLYSIS
IMPACT
FILMS

Journal

Trends in Chemistry cover
Trends in Chemistry
IF:
13.6
Papers:
827
Citations:
5.7K

Organization

No organization information available
Cited Papers

Cited Papers

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errJaeckering, Anna; Goettsch, Frederike; Scha''ffler, Moritz; Doerr, Mark; Bornscheuer, Uwe T.; Wei, Ren; Strodel, Birgit
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Rapid depolymerization of poly(ethylene terephthalate) thin films by a dual-enzyme system and its impact on material properties
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errTarazona, Natalia A.; Wei, Ren; Brott, Stefan; Pfaff, Lara; Bornscheuer, Uwe T.; Lendlein, Andreas; Machatschek, Rainhard
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Temporal and spatial evolution of enzymatic degradation of amorphous PET plastics
err2022-11-12
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errLippold, Holger; Kahle, Laura; Sonnendecker, Christian; Matysik, Joerg; Fischer, Cornelius
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Degradation Rates of Plastics in the Environment
err2020-02-03
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errChamas, Ali; Moon, Hyunjin; Zheng, Jiajia; Qiu, Yang; Tabassum, Tarnuma; Jang, Jun Hee; Abu-Omar, Mandi; Scott, Susannah L.; Suh, Sangwon
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UV Pretreatment Impairs the Enzymatic Degradation of Polyethylene Terephthalate
err2020-04-28
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errFalkenstein, Patricia; Graesing, Daniel; Bielytskyi, Pavlo; Zimmermann, Wolfgang; Matysik, Joerg; Wei, Ren; Song, Chen
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Merging Plastics, Microbes, and Enzymes: Highlights from an International Workshop
err2022-07-26
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errJimenez, Diego Javier; Oezturk, Basak; Wei, Ren; Bugg, Timothy D.; Amaya Gomez, Carol Viviana; Salcedo Galan, Felipe; Castro-Mayorga, Jinneth Lorena; Saldarriaga, Juan Fernando; Tarazona, Natalia Andrea
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Deep learning guided enzyme engineering of Thermobifida fusca cutinase for increased PET depolymerization
err2023-07-01
err6
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errMeng, Shuaiqi; Li, Zhongyu; Zhang, Peng; Contreras, Francisca; Ji, Yu; Schwaneberg, Ulrich
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Enzymatic depolymerization of polyester: Foaming as a pretreatment to increase specific surface area
err2024-08-29
err0
errOAAI
errAkanksha Patel; Allen C. Chang; Umer Abid; Christian Ayafor; Hsi‐Wu Wong; Dongming Xie; Margaret J. Sobkowicz
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