Metal- and additive-free cascade synthesis of diarylamines from biomass-derived feedstocks catalyzed by oxidized carbon

Mingze Yang

doi:10.1016/j.jcat.2026.117090

Metal- and additive-free cascade synthesis of diarylamines from biomass-derived feedstocks catalyzed by oxidized carbon

2026-07-31

0

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AI

M

Mingze Yang

A

Anna Lenarda

Y

Yushuai Sang

T

Takeharu Yoshii

K

Keigo Wakabayashi

L

Ligen Cha

J

Juho Helaja *

李

李永丹 (Yongdan Li) *

DOI：10.1016/j.jcat.2026.117090

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Abstract

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• Metal-free cascade synthesis of diarylamines from biomass substrates. • Up to 71% yield with stable activity over five catalytic cycles. • Acidic and quinoidic sites enable cascade and ODH steps. • Kinetics and DFT reveal radical-mediated regeneration by O2.

Metal- and additive-free cascade synthesis of diarylamines from biomass-derived feedstocks catalyzed by oxidized carbon

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