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Metal-nonmetal co-doping in Ti-MOF toward efficient photocatalytic nitrogen fixation
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DOI：10.1016/j.gce.2026.06.001.png)
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Abstract
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• A metal-nonmetal co-doping strategy is proposed to synergize electron transfer in MOFs. • Co and B co-doped NBM(Ti/Co) was synthesized via a hydrothermal method. • The electron-deficient B doping promotes the ligand-to-metal electron transfer. • The low-ionization-energy Co doping promotes the metal-to-metal electron transfer. • NBM(Ti/Co) yields an optimal NH3 production rate of 379.2 μmol g-1 h-1 under full spectrum.
Keywords:
Metal-organic framework
Metal-nonmetal Co-doping
Electron transfer pathway
Photocatalytic nitrogen fixation
Ammonia synthesis
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