arrow
Return

Multi-layered marble for hydrogel encapsulation

delete2026-03-23
delete0
delete
OA
AI
H
Hyeonjin Kim
S
Se Youn Jang
J
Ji Eun Lee
J
Jin Yoo
S
Syuji Fujii *
J
Jongkuk Ko *
S
Sanghyuk Wooh *
DOI:10.1038/s41467-026-70955-6delete
deleteOriginal
deleteOriginal request for help
deleteShare
deleteSave
Abstract

Abstract

En 中文
Hydrophobic skins on fruits play a crucial role in preventing dehydration and shielding against environmental stress. Inspired by this natural structure, hydrophobic encapsulation is widely employed to preserve the functionality and long-term stability of hydrogels. However, instability at the interface between hydrophobic shell and hydrogel remains a critical challenge. Here, we present a hydrogel encapsulation strategy to stabilize the incompatible interface using a concept of liquid marble, where liquid droplet is covered with hydrophobic particles. A uniform nonpolar liquid layer is first formed on the hydrogel surface through interfacial bridges with hydrophobic particles. A secondary hydrophobic particle layer is then deposited onto this liquid layer to prevent leakage, yielding a multi-layered marble (MLM) structure. This MLM-encapsulation is highly versatile, accommodating various hydrogels, liquids, and structural configurations. By maintaining hydrogel performance and functionality across diverse applications, MLM-encapsulation provides a universal and robust solution for overcoming the long-standing interfacial instability problem. Hydrogel encapsulation prevents dehydration, but maintaining interfacial stability with hydrophobic shells remains challenging. Here, the authors use a multi-layered marble strategy composed of two hydrophobic particle layers with sandwiched oil layer that stabilizes the interface.

Journal

Nature Communications cover
Nature Communications
IF:
15.7
Papers:
9.3W
Citations:
91.2W

Organization

C
chung-ang university
Scholars:
1.3K
Papers: 584
Citations: 0
O
Osaka Institute of Technology
Scholars:
807
Papers: 662
Citations: 472
K
korea institute of science and technology
Scholars:
2.1K
Papers: 769
Citations: 1
G
gachon university
Scholars:
2.0K
Papers: 1.2K
Citations: 0
researcher View more organizations