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Nitrogen radical-regulated reaction pathways for enhanced coal gasification in supercritical water
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DOI：10.1016/j.joei.2026.102682.png)
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Abstract
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• Urea boosts H2 yield from 8.10 to 10.70 mol/kg and carbon efficiency to 30.12%. • ·NH2 radicals from urea open aromatic rings of coal. • Nitrogen converts to liquid ammonia, enabling pollutant control and recovery. • Phenol is the key intermediate; its evolution correlates with gasification depth. • H2O serves as both reaction medium and primary H and O source for H2 and CO2.
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